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Page Title: Production and Removal of Samarium-149
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SAMARIUM AND OTHER FISSION PRODUCT POISONS
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Nuclear Physics and Reactor Theory Volume 2 of 2
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Samarium-149  Response  to  Reactor  Shutdown

DOE-HDBK-1019/2-93 SAMARIUM AND OTHER FISSION PRODUCT POISONS Reactor Theory (Nuclear Parameters) For  the  purpose  of  examining  the  behavior  of  samarium-149,  the  1.73  hour  half-life  of neodymium-149  is  sufficiently  shorter  than  the  53.1  hour  value  for  promethium-149  that  the promethium-149 may be considered as if it were formed directly from fission.  This assumption, and neglecting the small amount of promethium burnup, allows the situation to be described as follows. Rate of change of 149Pm = yield from fission - decay 149Pm concentration therefore: dNPm dt Pm  S fuel f f    lPm  NPm where: NPm = 149Pm concentration gPm = 149Pm fission yield lPm = decay constant for 149Pm Solving for the equilibrium value of promethium-149 gives the following. NPm(eq)                        Pm  S fuel f f lPm The rate of samarium-149 formation is described as follows. Rate of change of 149Sm = yield from fission + 149Pm decay - 149Sm burnup therefore: dNSm dt Sm  S fuel f f    lPm  NPm     NSm  s Sm a f where: NSm = 149Sm concentration gSm = 149Sm fission yield sa Sm = microscopic absorption cross section of 149Sm NP-03 Rev. 0 Page 44

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